Demonstration of high-order dispersion cancellation with an ultrahigh-efficiency sum-frequency correlator

We demonstrate dispersion cancellation of entangled photons for arbitrary spectral orders, generalizing Franson cancellation typically considered in second order alone. Employing ultrafast coincidence detection based on sum-frequency generation in a periodically poled lithium niobate waveguide with a record-high pair conversion efficiency of 10(-5), we verify cancellation of dispersion up to fifth order. Cancellation of odd-order phase is experimentally shown to require identical signal and idler dispersion coefficients, in contrast to even-order phase, which cancels with opposite signs. These results are especially important for future work on ultrabroadband biphotons.