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Updated: May 3, 2026

Stimulated Stokes and Antistokes Raman Scattering in Microspherical Whispering Gallery Mode Resonators
Published on: April 4, 2016
Coherent anti-Stokes Raman spectroscopy utilizing phase mismatched cascaded quadratic optical interactions in
Abstract:
We experimentally investigated the nonlinear optical interaction between the instantaneous four-wave mixing and the cascaded quadratic frequency conversion in commonly used nonlinear optical KTP and LiNbO3 with the aim of a possible background suppression of the non-resonant background in coherent anti-Stokes Raman scattering. The possibility of background-free heterodyne coherent anti-Stokes Raman scattering microspectroscopy is investigated at the interface formed by a liquid (isopropyl alcohol) and a nonlinear crystal (LiNbO3).
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