Related Experiment Video
Updated: May 2, 2026

An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
Published on: October 23, 2018
CITIUS: an infrared-extreme ultraviolet light source for fundamental and applied ultrafast science
C Grazioli1, C Callegari2, A Ciavardini3
1Laboratory of Quantum Optics, University of Nova Gorica, Nova Gorica, Slovenia.
Abstract:
We present the main features of CITIUS, a new light source for ultrafast science, generating tunable, intense, femtosecond pulses in the spectral range from infrared to extreme ultraviolet (XUV). The XUV pulses (about 10(5)-10(8) photons/pulse in the range 14-80 eV) are produced by laser-induced high-order harmonic generation in gas. This radiation is monochromatized by a time-preserving monochromator, also allowing one to work with high-resolution bandwidth selection. The tunable IR-UV pulses (10(12)-10(15) photons/pulse in the range 0.4-5.6 eV) are generated by an optical parametric amplifier, which is driven by a fraction of the same laser pulse that generates high order harmonics. The IR-UV and XUV pulses follow different optical paths and are eventually recombined on the sample for pump-probe experiments. We also present the results of two pump-probe experiments: with the first one, we fully characterized the temporal duration of harmonic pulses in the time-preserving configuration; with the second one, we demonstrated the possibility of using CITIUS for selective investigation of the ultra-fast dynamics of different elements in a magnetic compound.
Related Concept Videos
Ultraviolet and Visible (UV–Vis) Spectroscopy: Overview
Infrared (IR) Spectroscopy: Overview
Different compounds display unique properties due to their...
Atomic Absorption Spectroscopy: Radiation and Light Sources
Two common narrow-range 'line' sources used in AAS are hollow-cathode lamps (HCLs) and...
Total Internal Reflection Fluorescence Microscopy
IR Spectrometers
Fluorescence and Phosphorescence: Instrumentation

