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Friction through reversible jumps of surface atoms
O Y Fajardo1, Itay Barel, Michael Urbakh
1School of Chemistry, Tel Aviv University, 69978 Tel Aviv, Israel.
Summary
Surface atom motion significantly impacts nanoscopic friction, causing stick-slip behavior. This study reveals how atomic jumps influence friction and temperature dependence, explaining experimental observations.
Area of Science:
- Surface science
- Tribology
- Materials science
Background:
- Nanoscopic friction is crucial for understanding material wear and performance.
- Previous models often simplified the role of atomic motion in friction.
- Experimental friction force microscopy (FFM) shows complex temperature dependencies.
Purpose of the Study:
- To develop a microscopic model for nanoscopic friction.
- To investigate the role of thermally activated surface atom motion.
- To explain the nonmonotonic temperature dependence of friction observed in experiments.
Main Methods:
- Development of a microscopic model incorporating atomic jumps.
- Computational simulations of tip-sample interactions.
- Analysis of energy dissipation during atomic motion.
Main Results:
- Identified two competing processes governing stick-slip motion: jumps to the tip (inhibiting sliding) and jumps back to the sample (enabling sliding).
- Demonstrated that energy dissipated during reversible atomic jumps significantly contributes to friction.
- Showed a nonmonotonic dependence of friction on temperature, consistent with FFM experiments.
Conclusions:
- The proposed model provides a physical basis for microscopic instabilities in friction.
- Thermally activated surface atom motion is a key factor in nanoscopic friction.
- The model successfully explains experimental friction behaviors across various materials.
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