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Published on: August 2, 2019
Quantum critical fluctuations in the heavy fermion compound Ce(Ni0.935Pd0.065)₂Ge₂
C H Wang1, L Poudel, A E Taylor
1Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA. University of California, Irvine, CA 92697, USA.
This study investigates spin fluctuations in a heavy fermion compound near an antiferromagnetic quantum critical point. Alloy disorder may explain deviations from expected quantum critical point behavior.
Area of Science:
- Condensed Matter Physics
- Quantum Critical Phenomena
- Materials Science
Background:
- Heavy fermion compounds exhibit complex magnetic behavior.
- Quantum critical points (QCPs) are fascinating states where magnetic order is suppressed by quantum fluctuations.
- Understanding QCPs is crucial for developing new materials with exotic electronic properties.
Purpose of the Study:
- To investigate spin fluctuations in the heavy fermion compound Ce(Ni0.935Pd0.065)2Ge2.
- To study the behavior of this material near an antiferromagnetic (AF) quantum critical point (QCP).
- To explore the influence of alloy disorder on quantum critical phenomena.
Main Methods:
- Single crystal growth of Ce(Ni0.935Pd0.065)2Ge2.
- Measurements of electric resistivity and specific heat.
- Magnetic susceptibility and inelastic neutron scattering experiments.
Main Results:
- Observed power law behavior in resistivity and specific heat at low temperatures (T ≤ 1 K), consistent with a 3D itinerant AF QCP.
- Observed logarithmic temperature dependence in susceptibility and specific heat, and linear resistivity at intermediate temperatures (2 K ≤ T ≤ 10 K).
- Spin fluctuation correlation length, time, and staggered susceptibility remained finite, deviating from expected QCP divergence.
Conclusions:
- The material exhibits non-Fermi liquid behavior, indicative of proximity to a QCP.
- Deviations from expected QCP scaling suggest the significant role of alloy disorder.
- Alloy disorder may suppress the development of long-range correlations and influence the nature of quantum criticality.
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