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Related Experiment Video

Updated: Apr 18, 2026

Fabrication of Three-Dimensional Graphene-Based Polyhedrons via Origami-Like Self-Folding
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Fabrication of Three-Dimensional Graphene-Based Polyhedrons via Origami-Like Self-Folding

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Printing in three dimensions with graphene.

Esther García-Tuñon1, Suelen Barg, Jaime Franco

  • 1Centre for Advanced Structural Ceramics, Department of Materials, Imperial College London, London, SW7 2BP, UK.

Advanced Materials (Deerfield Beach, Fla.)
|January 22, 2015
PubMed
Summary

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Responsive graphene oxide sheets form networks ideal for 3D printing. These structures can be reduced to create lightweight, conductive, and elastic graphene materials.

Area of Science:

  • Materials Science
  • Nanotechnology
  • Polymer Science

Background:

  • Graphene oxide (GO) is a promising material due to its unique properties.
  • Developing GO-based materials for additive manufacturing requires careful control over rheological properties.
  • Achieving self-supporting structures in 3D printing with GO is challenging.

Purpose of the Study:

  • To develop responsive graphene oxide sheets for 3D printing applications.
  • To optimize the rheological properties of graphene oxide networks for direct write assembly.
  • To create ultra-light, conductive, and elastomeric graphene-only structures via post-processing.

Main Methods:

  • Formation of non-covalent networks using graphene oxide sheets.
  • Characterization of rheological properties, including shear thinning behavior and elastic shear modulus (G').
Keywords:
3D printingfunctionalizationgrapheneresponsive polymers

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  • Utilizing direct write assembly for 3D printing of the GO networks.
  • Post-processing via drying and thermal reduction to obtain graphene-only structures.

    • Main Results:

    • Graphene oxide sheets formed networks with optimal rheological properties for 3D printing.
    • The networks exhibited shear thinning behavior and a high elastic shear modulus (G'), enabling self-supporting 3D structures.
    • Post-processed structures were ultra-light, possessed restored electrical conductivity, and showed elastomeric behavior.

    Conclusions:

    • Responsive graphene oxide networks are suitable for 3D printing using direct write assembly.
    • The developed method allows for the creation of complex, self-supporting 3D structures.
    • Thermal reduction of printed GO structures yields advanced graphene materials with desirable functional properties.