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Enhanced Catalytic Efficiency of Pt Nanoparticles Supported on 3D Ordered Macro-/Mesoporous Ce0.6 Zr0.3 Y0.1 O2 for
Hamidreza Arandiyan1,2, Hongxing Dai3, Kemeng Ji3
1State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China.
Abstract:
Highly dispersed Pt nanoparticles supported on high-surface-area 3D ordered macroporous (3DOM) Ce0.6 Zr0.3 Y0.1 O2 (CZY) are synthesized via a bubbling cetyltrimethyl ammonium bromide/P123-assisted reduction route. The 1.1 wt% Pt/3DOM CZY catalyst shows supercatalytic activity for methane combustion, which is attributed to a higher oxygen adspecies amount, larger surface area, better low-temperature reducibility, and unique nanovoid-walled 3DOM structure.
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