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Synthesis of Zeolites Using the ADOR Assembly-Disassembly-Organization-Reassembly Route
Published on: April 3, 2016
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Synthesis of new zeolite structures.
Jiyang Li1, Avelino Corma, Jihong Yu
1State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun 130012, P. R. China. jihong@jlu.edu.cn.
Chemical Society Reviews
|March 6, 2015
Summary
Researchers are discovering new zeolites with unique structures for catalysis and separation. Recent synthetic strategies have yielded novel materials with complex pores and topologies.
Area of Science:
- Zeolite science
- Materials chemistry
- Porous materials
Background:
- Zeolites are crucial for catalysis and adsorption-separation.
- Developing new zeolites with novel structures is an ongoing scientific pursuit.
- Understanding zeolite formation is key to designing new materials.
Purpose of the Study:
- To review recent advances in the synthesis of new zeolite structures.
- To highlight synthetic strategies enabling the discovery of novel zeolites.
- To showcase the structural diversity of newly synthesized zeolites.
Main Methods:
- Utilizing pre-designed structure-directing agents.
- Employing heteroatom substitution in zeolite frameworks.
- Applying topotactic transformations for structural modification.
Main Results:
- Discovery of zeolites with hierarchical pores.
- Synthesis of zeolites with odd-ring numbers (11-, 15-rings).
- Creation of zeolites with extra-large pores (up to 30-rings), chiral pores, and complex topologies.
Conclusions:
- Recent synthetic strategies have significantly expanded the library of known zeolite structures.
- Novel zeolites with unprecedented pore architectures and compositions are now accessible.
- These advances promise new applications in catalysis and adsorption-separation.
