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Macroscopic discontinuous shear thickening versus local shear jamming in cornstarch
A Fall1, F Bertrand1, D Hautemayou1
1Laboratoire Navier (UMR CNRS 8205), Université Paris Est, 77420 Champs-sur-Marne, France.
Discontinuous shear thickening (DST) in cornstarch occurs when flow separates into distinct low-density flowing and high-density jammed regions. Local measurements reveal the flowing part is often shear thinning, not DST.
Area of Science:
- Rheology
- Material Science
- Soft Matter Physics
Background:
- Discontinuous shear thickening (DST) is a phenomenon where viscosity abruptly increases under shear stress.
- Understanding the microstructural origins of DST is crucial for predicting material behavior.
Purpose of the Study:
- To investigate the local flow dynamics during discontinuous shear thickening (DST) in cornstarch.
- To reconcile macroscopic DST observations with local rheological properties.
Main Methods:
- Combined macroscopic rheometry with local magnetic resonance imaging (MRI).
- Analyzed the coexistence of flowing and jammed regions in shear-thickened cornstarch.
Main Results:
- Macroscopic DST emerges only when flow separates into low-density flowing and high-density jammed regions.
- The local rheology within the flowing region is frequently shear thinning, not shear thickening.
- The observed stress jump in DST does not represent a high-viscosity branch of local rheology.
Conclusions:
- DST in cornstarch is driven by the formation of distinct flowing and jammed phases.
- Shear jamming limit, occurring below random close packing, explains the macroscopic stress jump.
- Local shear-thinning behavior in flowing regions challenges conventional understanding of DST mechanisms.
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