Piezo-phototronic Effect Enhanced UV/Visible Photodetector Based on Fully Wide Band Gap Type-II ZnO/ZnS Core/Shell
Satish C Rai1, Kai Wang1, Yong Ding2
1†Advanced Materials Research Institute, University of New Orleans, New Orleans, Louisiana 70148, United States.
This study presents a novel UV/visible photodetector using a ZnO/ZnS heterojunction nanowire array. The device exhibits enhanced performance through the piezo-phototronic effect, enabling detection of lower energy photons.
Area of Science:
- Materials Science
- Nanotechnology
- Optoelectronics
Background:
- Wide bandgap semiconductor heterojunctions are crucial for advanced photodetectors.
- ZnO and ZnS offer tunable electronic and optical properties.
- Type-II heterojunctions enable unique charge carrier dynamics.
Purpose of the Study:
- To fabricate a high-performance broadband UV/visible photodetector.
- To investigate the role of type-II heterojunctions in photon detection.
- To enhance photodetector performance using the piezo-phototronic effect.
Main Methods:
- Fabrication of ZnO/ZnS type-II heterojunction core/shell nanowire arrays.
- Characterization of the photodetector's response to UV and visible light.
- Analysis of the piezo-phototronic effect on charge carrier transport.
Main Results:
- Successful fabrication of a broadband UV/visible photodetector.
- Detection of photons with energies below the individual band gaps (2.2 eV).
- Three orders of magnitude change in relative responsivity due to the piezo-phototronic effect.
Conclusions:
- The ZnO/ZnS type-II heterojunction facilitates detection of lower energy photons.
- The piezo-phototronic effect significantly enhances photodetector performance.
- Demonstration of a prototype 3D core/shell nanowire array photodetector with improved capabilities.
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