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Updated: Apr 11, 2026

Methods of Ex Situ and In Situ Investigations of Structural Transformations: The Case of Crystallization of Metallic Glasses
Published on: June 7, 2018
Evidence for a Disordered Critical Point in a Glass-Forming Liquid
Ludovic Berthier1, Robert L Jack2
1Laboratoire Charles Coulomb, UMR 5221 CNRS-Université de Montpellier, 34095 Montpellier, France.
Abstract:
Using computer simulations of an atomistic glass-forming liquid, we investigate the fluctuations of the overlap between a fluid configuration and a quenched reference system. We find that large fluctuations of the overlap develop as temperature decreases, consistent with the existence of the random critical point that is predicted by effective field theories. We discuss the scaling of fluctuations near the presumed critical point, comparing the observed behavior with that of the random-field Ising model. We argue that this critical point directly reveals the existence of an interfacial tension between amorphous metastable states, a quantity relevant both for equilibrium relaxation and for nonequilibrium melting of stable glass configurations.
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