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A Hierarchical Particle-Shell Architecture for Long-Term Cycle Stability of Li2S Cathodes

Feixiang Wu1, Jung Tae Lee1, Feifei Fan2

  • 1School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.

Advanced Materials (Deerfield Beach, Fla.)
|August 26, 2015
PubMed

Keywords:
conversionlithium sulfidemechanical stabilitymultiscalesulfur

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In the region where two bulk phases meet, an intricate electric charge distribution arises due to charge transfer, ion adsorption, molecular orientation, and charge distortion. This complex distribution is commonly referred to as the electrical double layer.When a solid electrode interfaces with ions in an electrolyte solution, the speed of electron transfer dictates the rates of oxidation and reduction. The electrode acquires a charge through the escape of atoms into the solution as cations or...
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