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Oscillatory cellular patterns in three-dimensional directional solidification.

D Tourret1, J-M Debierre2, Y Song1

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Summary
This summary is machine-generated.

Microgravity experiments reveal synchronized cellular array oscillations during solidification. Phase-field simulations link these breathing modes to spacing stability limits in hexagonal structures.

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Area of Science:

  • Materials Science
  • Solidification Physics
  • Microgravity Research

Background:

  • Directional solidification in microgravity minimizes convection, enabling observation of cellular and dendritic array formation.
  • In situ observations revealed oscillatory breathing modes in cellular arrays within a narrow parameter range (25-125 min period).
  • These oscillations were spatially uncorrelated over long distances but synchronized in ordered regions.

Purpose of the Study:

  • To investigate the mechanism behind oscillatory breathing modes in 3D cellular arrays during microgravity solidification.
  • To correlate observed oscillations with the stability of hexagonal cellular array structures.
  • To compare experimental findings with quantitative phase-field simulations.

Main Methods:

  • Phase-field simulations of three-dimensional cellular array solidification.
  • Analysis of microgravity directional solidification experiments using transparent alloys.
  • Quantitative comparison of simulated and experimental oscillation periods and spatial ordering.

Main Results:

  • Oscillatory behavior is linked to a stability limit in hexagonal cellular array spacing, creating a gap in stable spacings.
  • A sustained oscillatory regime emerges near this gap, with periods matching experimental observations.
  • Simulations show long-range coherence is achievable with perfect initial conditions, but disorder prevails with realistic noisy inputs, similar to experiments.

Conclusions:

  • The study identifies a critical link between array spacing stability and oscillatory breathing modes in microgravity solidification.
  • Phase-field modeling successfully reproduces experimentally observed phenomena, validating the proposed mechanism.
  • Global disorder in experiments and simulations arises from initial conditions and tip-splitting events, contrasting with ordered thin-sample results.