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Updated: Mar 24, 2026

All-electronic Nanosecond-resolved Scanning Tunneling Microscopy: Facilitating the Investigation of Single Dopant Charge Dynamics
Published on: January 19, 2018
Real-Time Probing of Electron Dynamics Using Attosecond Time-Resolved Spectroscopy
Krupa Ramasesha1,2, Stephen R Leone1,3,4, Daniel M Neumark1,4
1Department of Chemistry, University of California, Berkeley, California 94720;
Attosecond science uses ultrashort pulses to observe electron motion in atoms, molecules, and solids. This enables real-time studies of ionization, charge migration, and electron dynamics in materials.
Area of Science:
- Attosecond science
- Quantum dynamics
- Ultrafast spectroscopy
Background:
- Attosecond science enables direct observation of electron dynamics.
- Isolated attosecond pulses are key tools for studying ultrafast phenomena.
Purpose of the Study:
- To review recent attosecond measurements and their insights into electron dynamics.
- To highlight applications in gases and solid-state systems.
Main Methods:
- Attosecond photoelectron and photoion spectroscopy in atoms and molecules.
- Attosecond transient absorption spectroscopy (ATAS) in atoms and solids.
Main Results:
- Observed strong-field tunneling ionization and photoemission delays in atoms.
- Revealed ultrafast intramolecular charge migration in molecules.
- Measured bulk electron dynamics in solids, including insulator-to-metal transitions and carrier interactions.
Conclusions:
- Attosecond science provides unprecedented real-time insights into electron dynamics.
- Applications span from atomic and molecular physics to condensed matter physics.
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