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Updated: Mar 23, 2026

Methods of Ex Situ and In Situ Investigations of Structural Transformations: The Case of Crystallization of Metallic Glasses
Published on: June 7, 2018
Hall effect in quantum critical charge-cluster glass.
Jie Wu1, Anthony T Bollinger1, Yujie Sun2
1Condensed Matter Physics and Materials Science Division, Brookhaven National Laboratory, Upton, NY 11973-5000;
Quantum critical fluctuations in La2-xSrxCuO4 (LSCO) were observed via Hall resistance anomalies. These fluctuations compete with superconductivity, highlighting a complex interplay near the quantum critical point.
Area of Science:
- Condensed Matter Physics
- Materials Science
Background:
- Cuprates exhibit a quantum phase transition from insulating to d-wave superconducting states upon doping.
- The precise nature of this transition and the insulating state remains a subject of intense scientific debate.
Purpose of the Study:
- Investigate the Hall effect in La2-xSrxCuO4 (LSCO) near the quantum critical point (x ~ 0.06).
- Characterize quantum critical behavior and its relationship with superconductivity.
Main Methods:
- Studied Hall resistance in LSCO samples doped near the quantum critical point.
- Utilized a combinatorial LSCO library with extremely fine Sr content steps (Δx ~ 0.00008) to analyze doping dependence.
- Applied magnetic fields to suppress superconductivity and observe its effect on quantum charge fluctuations.
Main Results:
- Observed dramatic fluctuations in Hall resistance below ~1.5 K, increasing with further cooling, indicative of quantum critical behavior.
- Found that quantum charge fluctuations diminish with the emergence of superconductivity.
- Demonstrated that these fluctuations can be restored by suppressing superconductivity with a magnetic field.
Conclusions:
- Quantum charge fluctuations and superconductivity in LSCO exhibit a competitive relationship for the ground state.
- The findings provide critical insights into the complex phase diagram of cuprate superconductors near their quantum critical point.
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