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Thermal rectification and negative differential thermal conductance in harmonic chains with nonlinear system-bath
Yi Ming1, Hui-Min Li2, Ze-Jun Ding3
1School of Physics and Material Science, Anhui University, Hefei, Anhui 230601, People's Republic of China.
This study demonstrates thermal rectification and negative differential thermal conductance in harmonic chains by incorporating nonlinear system-bath coupling. The findings reveal how coupling strength influences phonon transport and rectification direction.
Area of Science:
- Condensed Matter Physics
- Statistical Mechanics
- Nanoscale Heat Transfer
Background:
- Understanding heat flow in nanoscale systems is crucial for thermal management.
- Previous studies primarily focused on linear system-bath coupling.
- Recent experiments highlight the importance of nonlinear system-bath interactions.
Purpose of the Study:
- To investigate thermal rectification and negative differential thermal conductance in harmonic chains.
- To explore the effects of nonlinear system-bath coupling on heat transport.
- To analyze the influence of coupling strength on phonon transport mechanisms.
Main Methods:
- Utilized the generalized Caldeira-Leggett model for heat flow analysis.
- Incorporated nonlinear system-bath coupling, deviating from traditional linear models.
- Studied harmonic chains with asymmetric nonlinear couplings.
Main Results:
- Achieved thermal rectification and negative differential thermal conductance with asymmetric nonlinear couplings.
- Observed enhanced heat current under weak linear coupling due to nonlinear-induced multiphonon processes.
- Found that strong linear coupling leads to umklapp processes dominating, suppressing heat current and reversing rectification direction.
Conclusions:
- Nonlinear system-bath coupling is a key factor in realizing thermal rectification and negative differential thermal conductance.
- The strength of linear coupling critically determines the phonon transport mechanisms and the direction of thermal rectification.
- This work provides insights into controlling heat flow at the nanoscale through engineered system-bath interactions.
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