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    We report highly conductive and transparent electrodes made from DMSO-doped poly(3,4-ethylenedioxythiophene):poly(4-styrenesulfonate) (PEDOT:PSS) thin films for terahertz (THz) applications.

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    Area of Science:

    • Materials Science
    • Condensed Matter Physics
    • Optoelectronics

    Background:

    • Transparent conductive films are crucial for optoelectronic devices.
    • Poly(3,4-ethylenedioxythiophene):poly(4-styrenesulfonate) (PEDOT:PSS) is a promising material for transparent electrodes.
    • Terahertz (THz) frequencies present unique challenges for electrode materials.

    Purpose of the Study:

    • To investigate the use of DMSO-doped PEDOT:PSS thin films as transparent electrodes for THz applications.
    • To analyze the relationship between film thickness, DMSO doping, and electrode properties.
    • To evaluate the THz transmittance and electrical conductivity of the developed electrodes.

    Main Methods:

    • Fabrication of PEDOT:PSS thin films using spin coating.
    • Doping of PEDOT:PSS films with varying concentrations of Dimethyl sulfoxide (DMSO).
    • Characterization of film thickness, surface morphology, electrical conductivity, and THz transmittance.

    Main Results:

    • Achieved a maximum electrical conductivity of 5078 S/cm for a 52 nm single-layer film.
    • Obtained a maximum transmittance of 83.5% at 1.22 THz.
    • Demonstrated continuous tunability and electrical controllability using a novel blue-phase liquid crystal THz modulator.

    Conclusions:

    • DMSO-doped PEDOT:PSS thin films are effective transparent electrodes for THz frequencies.
    • Optimized doping and film thickness enhance conductivity and transmittance.
    • The developed materials are suitable for advanced THz modulation applications.