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Updated: Mar 20, 2026

Quantitative Atomic-Site Analysis of Functional Dopants/Point Defects in Crystalline Materials by Electron-Channeling-Enhanced Microanalysis
Published on: May 10, 2021
Orbital-exchange and fractional quantum number excitations in an f-electron metal, Yb₂Pt₂Pb
L S Wu1, W J Gannon2, I A Zaliznyak3
1Department of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794, USA. Condensed Matter Physics and Materials Science Division, Brookhaven National Laboratory, Upton, NY 11973, USA. Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.
Abstract:
Exotic quantum states and fractionalized magnetic excitations, such as spinons in one-dimensional chains, are generally expected to occur in 3d transition metal systems with spin 1/2. Our neutron-scattering experiments on the 4f-electron metal Yb2Pt2Pb overturn this conventional wisdom. We observe broad magnetic continuum dispersing in only one direction, which indicates that the underlying elementary excitations are spinons carrying fractional spin-1/2. These spinons are the emergent quantum dynamics of the anisotropic, orbital-dominated Yb moments. Owing to their unusual origin, only longitudinal spin fluctuations are measurable, whereas the transverse excitations such as spin waves are virtually invisible to magnetic neutron scattering. The proliferation of these orbital spinons strips the electrons of their orbital identity, resulting in charge-orbital separation.
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