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Updated: Mar 17, 2026

An Analog Macroscopic Technique for Studying Molecular Hydrodynamic Processes in Dense Gases and Liquids
Published on: December 4, 2017
Field-induced superdiffusion and dynamical heterogeneity
Giacomo Gradenigo1,2, Eric Bertin1,2, Giulio Biroli3,4
1Université Grenoble Alpes, LIPHY, F-38000 Grenoble, France.
Abstract:
By analyzing two kinetically constrained models of supercooled liquids we show that the anomalous transport of a driven tracer observed in supercooled liquids is another facet of the phenomenon of dynamical heterogeneity. We focus on the Fredrickson-Andersen and the Bertin-Bouchaud-Lequeux models. By numerical simulations and analytical arguments we demonstrate that the violation of the Stokes-Einstein relation and the field-induced superdiffusion observed during a long preasymptotic regime have the same physical origin: while a fraction of probes do not move, others jump repeatedly because they are close to local mobile regions. The anomalous fluctuations observed out of equilibrium in the presence of a pulling force ε,σ_{x}^{2}(t)=〈x_{ε}^{2}(t)〉-〈x_{ε}(t)〉^{2}∼t^{3/2}, which are accompanied by the asymptotic decay α_{ε}(t)∼t^{-1/2} of the non-Gaussian parameter from nontrivial values to zero, are due to the splitting of the probes population in the two (mobile and immobile) groups and to dynamical correlations, a mechanism expected to happen generically in supercooled liquids.
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