Midrefractive Dielectric Modulator for Broadband Unidirectional Scattering and Effective Radiative Tailoring in the...

Nanoantennas have found many applications in ultrasmall sensors, single-molecule detection, and all-optical communication. Conventional nanoantennas are based on noble-metal plasmonic structures, but suffer from large ohmic loss and only possess dipolar plasmon modes. This has driven an intense search for all-dielectric materials beyond noble metals. Here, we propose midrefractive nanospheres as a novel all-dielectric material to realize broadband unidirectional radiation and effective radiative tailoring in the visible region. Midrefractive all-dielectric materials such as boron nanospheres possess broad and overlapping electric and magnetic dipole modes. The internal interaction between these two modes can route the radiation almost on the one side covering the whole visible range. Unlike the elaborate design in plasmonic nanostructures to obtain strong coupled broad and narrow modes, the bright mode in boron nanospheres is intrinsic, independent, and easily coupled with adjacent narrow modes. So the strong interaction in boron-based heterodimer is able to realize an independent and precise tailoring of the radiant and subradiant states by simply changing the particle sizes, respectively. Our findings imply midrefractivity materials like boron are excellent building blocks to support electromagnetic coupling operation in nanoscale devices, which will lead to a variety of emerging applications such as nanoantennas with directing exciton emission, ultrasensitive nanosensors, or even potential new construction of photonic metamaterials.