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Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
Precise and Accurate Measurements of Strong-Field Photoionization and a Transferable Laser Intensity Calibration
W C Wallace1,2, O Ghafur1,2, C Khurmi1,2
1ARC Centre of Excellence for Coherent X-Ray Science, Griffith University, Brisbane, Queensland 4111, Australia.
Researchers accurately measured ionization yields for argon, krypton, and xenon using a novel calibration standard for strong laser fields. This breakthrough in attosecond science provides crucial data for atomic and molecular ionization studies.
Area of Science:
- Atomic and Molecular Physics
- Attosecond Science
- Strong Field Physics
Background:
- Accurate ionization yield data are crucial for understanding atomic and molecular processes in strong laser fields, particularly in attosecond science.
- Currently, reliable data are primarily available only for atomic hydrogen, limiting broader research.
- Noble gas atoms like argon, krypton, and xenon are widely studied but lack precise ionization yield benchmarks.
Purpose of the Study:
- To present percent-level accurate measurements of ionization yields for argon, krypton, and xenon.
- To establish a transferable calibration standard for laser peak intensity based on these measurements.
- To provide benchmark data for validating theoretical models of strong-field ionization in noble gases.
Main Methods:
- Utilizing a strong laser field regime common in attosecond science.
- Calibrating measurements using atomic hydrogen (H) as a reference.
- Developing a simple reference curve for deriving a laser peak intensity calibration standard.
Main Results:
- Achieved percent-level accuracy for ionization yield measurements in argon, krypton, and xenon.
- Derived a laser peak intensity calibration standard accurate to 1.3%.
- The calibration standard is transferable and based on a simple reference curve.
Conclusions:
- The study provides the first percent-level accurate ionization yield data for common noble gases.
- A reliable and transferable laser intensity calibration standard is now available for attosecond science.
- These findings offer essential benchmarks for refining theoretical models of atomic ionization, including the single-active electron approximation.
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