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Published on: March 24, 2019
A novel type of splayed ferromagnetic order observed in Yb2Ti2O7
A Yaouanc1,2, P Dalmas de Réotier1,2, L Keller3
1Université Grenoble Alpes, INAC-PHELIQS, F-38000 Grenoble, France.
Researchers observed magnetic Bragg reflections in Ytterbium Titanate (Yb2Ti2O7) using neutron powder diffraction. This pyrochlore insulator exhibits a splayed ferromagnet structure, distinct from its sibling compound Yb2Sn2O7.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Magnetism
Background:
- The pyrochlore insulator Ytterbium Titanate (Yb2Ti2O7) has been a subject of intense research for over 15 years.
- Previous neutron diffraction studies yielded conflicting results regarding magnetic Bragg reflections at low temperatures.
Purpose of the Study:
- To resolve conflicting experimental data on the magnetic structure of Yb2Ti2O7.
- To definitively observe and characterize magnetic Bragg reflections in Yb2Ti2O7 at millikelvin temperatures.
Main Methods:
- Neutron powder diffraction experiments were conducted at an ultra-low temperature of 60 mK.
- Representation theory was employed to analyze the observed magnetic diffraction pattern.
Main Results:
- The study successfully observed magnetic Bragg reflections in Yb2Ti2O7, confirming its magnetic ordering.
- Yb2Ti2O7 is identified as a splayed ferromagnet, similar to Yb2Sn2O7, indicated by a positive Curie-Weiss temperature.
- A key difference was found in the magnetic moment configuration: Yb2Ti2O7 exhibits an all-in-all-out arrangement, unlike the two-in-two-out configuration in Yb2Sn2O7.
Conclusions:
- The findings provide a clear experimental picture of the magnetic properties of Yb2Ti2O7.
- The distinct magnetic structure of Yb2Ti2O7 compared to Yb2Sn2O7 offers new insights into pyrochlore magnetism.
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