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In scanning tunnelling spectroscopy (STS), quantum effects cause current granularity, limiting energy resolution. This study demonstrates this quantum limit at 15 mK, impacting STS precision.

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Area of Science:

  • Quantum physics
  • Condensed matter physics
  • Surface science

Background:

  • Scanning tunnelling spectroscopy (STS) typically models tunnelling current as continuous.
  • At low temperatures, single-charge charging energy can exceed thermal energy, making current granularity significant.
  • The tunnel junction's capacitance couples tunnelling electrons to the electromagnetic environment, introducing noise.

Purpose of the Study:

  • To investigate the quantum limit of tunnelling current in STS.
  • To demonstrate that current granularity, mediated by junction capacitance, is a key factor in STS energy resolution.
  • To experimentally validate the P(E)-theory as the energy resolution function in this quantum regime.

Main Methods:

  • Utilized a scanning tunnelling microscope operated at an ultra-low temperature of 15 mK.
  • Employed superconducting aluminium as both the tip and sample material to enhance the quantum effects.
  • Analyzed the tunnelling current to identify and quantify the impact of quantum granularity and environmental noise.

Main Results:

  • Confirmed operation within the quantum limit where current granularity is non-negligible.
  • Showcased that the electromagnetic environment, mediated by junction capacitance, acts as a significant noise source.
  • Observed that the effect is most pronounced in superconducting systems, as predicted.

Conclusions:

  • The granularity of tunnelling current in the quantum limit fundamentally determines the ultimate energy resolution in STS.
  • The P(E)-theory accurately describes the probability of energy exchange between tunnelling electrons and the environment, serving as the energy resolution function.
  • Experimental validation at 15 mK with superconducting materials provides strong evidence for these quantum effects in STS.