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Innovation in Layer-by-Layer Assembly.

Joseph J Richardson1,2, Jiwei Cui1, Mattias Björnmalm1

  • 1ARC Centre of Excellence in Convergent Bio-Nano Science and Technology, and the Department of Chemical and Biomolecular Engineering, The University of Melbourne , Parkville, Victoria 3010, Australia.

Chemical Reviews
|December 15, 2016
PubMed
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Layer-by-layer assembly advances nanoscale film creation for functional materials. This review covers conventional, unconventional, and quasi-layer-by-layer assembly techniques, plus characterization methods, guiding future innovation.

Area of Science:

  • Materials Science
  • Nanotechnology
  • Surface Chemistry

Background:

  • Layer-by-layer (LbL) assembly has been a key method for nanoscale film fabrication for over 50 years.
  • Innovations in materials, assembly technologies, and characterization have driven growing interest in LbL assembly.
  • LbL assembly is crucial for developing functional materials across diverse scientific and industrial fields.

Purpose of the Study:

  • To review and detail innovations in layer-by-layer assembly, encompassing past, present, and future developments.
  • To highlight conventional and unconventional assembly approaches, including hybrid materials and advanced techniques.
  • To discuss the impact of quasi-layer-by-layer assembly and the importance of characterization methods.

Main Methods:

  • Exploration of conventional and early layer-by-layer assembly techniques.

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  • Review of unconventional methods such as inorganic/organic hybrids, cell/tissue assembly, stereocomplexation, patterning, and dip-pen lithography.
  • Discussion of quasi-layer-by-layer assembly for single-step film formation and relevant characterization techniques.

    • Main Results:

    • Identification of renewed interest in conventional layer-by-layer assembly methods.
    • Detailed overview of emerging unconventional assembly strategies and their applications.
    • Introduction and analysis of quasi-layer-by-layer assembly as a streamlined fabrication approach.
    • Emphasis on the critical role of characterization in advancing layer-by-layer assembly.

    Conclusions:

    • Layer-by-layer assembly continues to evolve, with significant innovations in both established and novel techniques.
    • Quasi-layer-by-layer assembly offers a promising pathway for efficient film fabrication.
    • Continued development in characterization methods is essential for the progress of nanoscale film assembly.