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Two-Dimensional Fluorinated Graphene: Synthesis, Structures, Properties and Applications.

Wei Feng¹, Peng Long¹, Yiyu Feng¹

¹School of Materials Science and Engineering Tianjin University Tianjin 300072 P.R China; Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) Tianjin 300072 P.R China; Key Laboratory of Advanced Ceramics and Machining Technology Ministry of Education Tianjin 300072 P.R China; Tianjin Key Laboratory of Composite and Functional Materials Tianjin 300072 P.R China.

Advanced Science (Weinheim, Baden-Wurttemberg, Germany)

|December 17, 2016

Summary

Fluorinated graphene offers tunable properties through controlled carbon-fluorine (C-F) bonds. This review details synthesis, properties, and applications of fluorinated graphene, highlighting future challenges.

Keywords:

C–F bonds F/C ratio fluorinated graphene fluorographene

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Area of Science:

Materials Science
Nanotechnology
Chemistry

Background:

Fluorinated graphene is a significant derivative of graphene.
It possesses a unique two-dimensional structure, wide bandgap, and high stability.
Its properties stem from its nanostructure and carbon-fluorine (C-F) bonds.

Purpose of the Study:

To extensively review recent advancements in fluorinated graphene synthesis and C-F bonding.
To present the optical, electrical, electronic, electrochemical, and biological properties.
To discuss potential applications and future challenges.

Main Methods:

Review of direct fluorination and exfoliation methods for synthesis.
Analysis of various C-F bond types (covalent, semi-ionic, ionic) and tunable F/C ratios.
Comprehensive discussion of structure-property relationships.

Main Results:

Fluorinated graphene exhibits diverse C-F bond configurations and tunable F/C ratios.
Properties like opened bandgap, high stability, dispersibility, semiconducting/insulating nature, and altered thermal/mechanical characteristics are observed.
Optimized C-F bonding enables applications in energy devices, bio-interfaces, sensors, and amphiphobic surfaces.

Conclusions:

Controlling C-F bonding and F/C ratios is crucial for tailoring fluorinated graphene properties.
Significant potential exists for energy conversion/storage, bioapplications, and sensing.
Further research is needed on synthetic methods and precise C-F bond characterization.