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Published on: May 10, 2021
Candidate Elastic Quantum Critical Point in LaCu_{6-x}Au_{x}
L Poudel1,2, A F May3, M R Koehler4
1Department of Physics & Astronomy, University of Tennessee, Knoxville, Tennessee 37966, USA.
Abstract:
The structural properties of LaCu_{6-x}Au_{x} are studied using neutron diffraction, x-ray diffraction, and heat capacity measurements. The continuous orthorhombic-monoclinic structural phase transition in LaCu_{6} is suppressed linearly with Au substitution until a complete suppression of the structural phase transition occurs at the critical composition x_{c}=0.3. Heat capacity measurements at low temperatures indicate residual structural instability at x_{c}. The instability is ferroelastic in nature, with density functional theory calculations showing negligible coupling to electronic states near the Fermi level. The data and calculations presented here are consistent with the zero temperature termination of a continuous structural phase transition suggesting that the LaCu_{6-x}Au_{x} series hosts an elastic quantum critical point.
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