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Updated: Mar 9, 2026

Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
Strong-field ionization of clusters using two-cycle pulses at 1.8 μm
Bernd Schütte1, Peng Ye1, Serguei Patchkovskii2
1Department of Physics, Imperial College London, South Kensington Campus, London SW7 2AZ, UK.
Intense laser pulses interacting with rare-gas clusters generate high-energy electrons. Longer laser wavelengths (1.8 μm) significantly boost electron energies compared to shorter wavelengths (800 nm).
Area of Science:
- Plasma physics
- Atomic and molecular physics
- Laser-driven particle acceleration
Background:
- Previous studies focused on longer laser pulses (many optical cycles) interacting with nanoscale particles.
- Investigations typically used near-infrared to X-ray laser pulses.
Purpose of the Study:
- To explore strong-field ionization of rare-gas clusters using ultrashort, two-cycle 1.8 μm laser pulses.
- To access a new interaction regime where electron dynamics are laser-dominated and atomic motion is negligible.
Main Methods:
- Irradiation of rare-gas clusters (10^3–10^5 atoms) with two-cycle 1.8 μm laser pulses at an intensity of 1 × 10^15 W/cm^2.
- Comparison with experiments using 800 nm laser pulses of similar intensity and duration.
- Analysis of emitted electron energies and emission directionality.
Main Results:
- Observation of fast electron emission exceeding 3 keV at 1.8 μm, significantly higher than electrons below 500 eV at 800 nm.
- Preferential emission of energetic electrons along the laser polarization direction.
- Evidence of an electron rescattering plateau in addition to direct emission.
Conclusions:
- Ultralong wavelength laser pulses enable a new regime for generating energetic electrons from rare-gas clusters.
- Scaling to longer wavelengths is predicted to produce highly directional, energetic electron currents on femtosecond timescales.
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