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High-Performance All-Inorganic Solid-State Sodium-Sulfur Battery.

Jie Yue1,2, Fudong Han1, Xiulin Fan1

  • 1Department of Chemical and Biomolecular Engineering, University of Maryland , College Park, Maryland 20742, United States.

ACS Nano
|May 2, 2017
PubMed
Summary
This summary is machine-generated.

This study introduces a novel nanocomposite cathode for all-inorganic solid-state sodium-sulfur batteries (ASSBs). The new cathode significantly enhances cycling and rate performance, paving the way for practical energy storage applications.

Keywords:
all-inorganicall-solid-stateelectrode designnanocompositesodium−sulfur battery

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-inorganic solid-state sodium-sulfur batteries (ASSBs) offer safe and high-energy stationary storage.
  • Current ASSBs suffer from poor performance due to high interfacial resistance and insufficient triple-phase contact.

Purpose of the Study:

  • To develop an innovative cathode material to overcome interfacial challenges in ASSBs.
  • To improve the cycling and rate performance of ASSBs for practical applications.

Main Methods:

  • Fabrication of a Na3PS4-Na2S-C nanocomposite cathode.
  • Utilizing Na3PS4 as both a solid electrolyte and active material (catholyte).
  • Incorporating nanosized Na2S to enhance capacity and conductivity.

Main Results:

  • The nanocomposite cathode achieved a high initial discharge capacity of 869.2 mAh g-1 at 50 mA g-1.
  • Demonstrated excellent cycling stability and rate capabilities at 60 °C.
  • Achieved superior electrode/electrolyte interfacial contact due to a two-phase reaction mechanism.

Conclusions:

  • The developed Na3PS4-nanosized Na2S-carbon nanocomposite cathode represents a significant advancement for high-performance ASSBs.
  • This approach effectively addresses interfacial resistance, leading to record-breaking performance.
  • The findings pave the way for practical stationary energy storage solutions using ASSBs.