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Harmonium: An Ultrafast Vacuum Ultraviolet Facility.

Christopher A Arrell1, José Ojeda2, Luca Longetti2

  • 1Laboratory of Ultrafast Spectroscopy and Lausanne Centre for Ultrafast Science (LACUS) ISIC Station 6 Ecole Polytechnique Fédérale de Lausanne (EPFL) CH-1015 Lausanne;,

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|June 4, 2017
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Summary

Harmonium, a new vacuum ultraviolet photon source, enables advanced spectroscopy techniques with high resolution and flux. This facility supports ultrafast science research in Switzerland.

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Area of Science:

  • Ultrafast Science
  • Photon Source Development
  • Spectroscopy

Background:

  • The Lausanne Centre for Ultrafast Science (LACUS) developed Harmonium, a novel vacuum ultraviolet (VUV) photon source.
  • Existing infrastructure required enhancement for advanced spectroscopic studies.

Purpose of the Study:

  • To establish a versatile VUV photon source for ultrafast and steady-state spectroscopy.
  • To provide high energy and temporal resolution capabilities for diverse sample types.
  • To complement existing Swiss research facilities and advance ultrafast science.

Main Methods:

  • High harmonic generation (HHG) for VUV photon production (20-110 eV).
  • A pulse-preserving monochromator offering high energy (70 meV) or temporal (40 fs) resolution.
  • Three specialized endstations for liquids, solids (ARPES), and gas-phase molecules/clusters.

Main Results:

  • Harmonium delivers high photon flux (10^11 photons/sec at 38 eV) and high repetition rate (up to 15 kHz).
  • Commissioned endstations facilitate photoelectron spectroscopy (PES), angular resolved PES (ARPES), and coincidence PES/PIS.
  • The source provides tunable energy and time resolution for advanced material and molecular studies.

Conclusions:

  • Harmonium significantly enhances capabilities for ultrafast spectroscopy in Switzerland.
  • The facility supports a broad range of scientific investigations, from condensed matter to molecular dynamics.
  • It strengthens Switzerland's position in global ultrafast and X-ray science research.