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Fabrication of Spatially Confined Complex Oxides
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Electronic Band Alignment at Complex Oxide Interfaces Measured by Scanning Photocurrent Microscopy.

J H Yoon1, H J Jung1, J T Hong1

  • 1Department of Physics and Department of Energy Systems Research, Ajou University, Suwon, 16499, Korea.

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|June 21, 2017
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Summary

Researchers investigated the electronic band alignment at an Al2O3/SrTiO3 heterointerface forming a two-dimensional electron gas (2DEG). Scanning photocurrent microscopy revealed unique gate responses, enabling valence band offset determination.

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Area of Science:

  • Materials Science
  • Condensed Matter Physics
  • Semiconductor Heterostructures

Background:

  • The Al2O3/SrTiO3 interface is crucial for forming two-dimensional electron gases (2DEGs).
  • Understanding band alignment is essential for device performance and novel electronic applications.
  • Scanning Photocurrent Microscopy (SPCM) is a powerful tool for probing interfacial electronic properties.

Purpose of the Study:

  • To investigate the band alignment at the Al2O3/SrTiO3 heterointerface.
  • To characterize the electronic properties of the 2DEG formed at this interface.
  • To determine the valence band offset using SPCM in an electrolyte-gated environment.

Main Methods:

  • Utilized scanning photocurrent microscopy (SPCM) with a focused UV laser.
  • Employed an electrolyte-gated environment for tunable device characteristics.
  • Performed transport measurements to analyze gate-dependent conductance.

Main Results:

  • SPCM on bare SrTiO3 showed p-type behavior, collecting photogenerated electrons.
  • SPCM on the 2DEG device exhibited hole carrier collection, indicating unique interfacial behavior.
  • Gate-dependent conductance measurements confirmed n-type switching behavior of the 2DEG.
  • Observed unique SPCM gate responses in 2DEG devices, distinct from conventional semiconductors.

Conclusions:

  • The study successfully determined the electronic band alignment at the Al2O3/SrTiO3 heterointerface.
  • SPCM in an electrolyte-gated setup is effective for investigating 2DEG properties and band offsets.
  • The findings provide critical insights into the behavior of 2DEGs at oxide interfaces.