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Wavevector-Selective Nonlinear Plasmonic Metasurfaces.

Kuang-Yu Yang1, Ruggero Verre2, Jérémy Butet1

  • 1Nanophotonics and Metrology Laboratory, Swiss Federal Institute of Technology Lausanne (EPFL) , 1015 Lausanne, Switzerland.

Nano Letters
|August 23, 2017
PubMed
Summary
This summary is machine-generated.

We demonstrated that plasmonic metasurfaces with tilted gold nanopillars act as wavevector-selective nonlinear optical components. Their nonlinear response strongly depends on the angle of incidence, enabling directional nonlinear mirrors.

Keywords:
Metamaterialsdirectionalitynonlinear optical materialnonlinear plasmonicssecond harmonic generation

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Area of Science:

  • Photonics and Optics
  • Materials Science
  • Nonlinear Optics

Background:

  • Electromagnetic metasurfaces offer novel functionalities for ultrathin optical components.
  • Strong nonlinear responses and angular selectivity are key for advanced optical designs.
  • Plasmonic metasurfaces provide a versatile platform for manipulating light-matter interactions.

Purpose of the Study:

  • To investigate optical second harmonic generation (SHG) from plasmonic metasurfaces.
  • To explore the wavevector-selective nonlinear response of metasurfaces with tilted nanopillars.
  • To demonstrate the potential for designing directional nonlinear optical devices.

Main Methods:

  • Fabrication of plasmonic metasurfaces composed of aligned gold nanopillars with an out-of-plane tilt.
  • Utilized a flexible nonlinear Fourier microscope for experimental investigation.
  • Performed computational modeling to analyze the nonlinear optical response.

Main Results:

  • The metasurfaces exhibit wavevector-selective nonlinear behavior, with SHG dependent on excitation beam polarization, wavelength, and incidence direction.
  • A significant variation (nearly two orders of magnitude) in nonlinear response was observed by altering the incidence angle.
  • The metasurfaces function as directional nonlinear mirrors.

Conclusions:

  • Tilted plasmonic metasurfaces act as efficient wavevector-selective nonlinear optical elements.
  • The angular dependence of the nonlinear response opens new possibilities for directional optical control.
  • These findings pave the way for novel directional meta-mirrors in the nonlinear optical regime.