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Tailoring Ink-Substrate Interactions via Thin Polymeric Layers for High-Resolution Printing.

Aleksander Matavž1,2, Vid Bobnar1,2, Barbara Malič1,2

  • 1Jožef Stefan Institute , Jamova cesta 39, 1000 Ljubljana, Slovenia.

Langmuir : the ACS Journal of Surfaces and Colloids
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Summary

Controlling surface properties with nanometer-thick polymer layers improves inkjet printing resolution and feature stability. Thermal decomposition of poly(methyl methacrylate) (PMMA) offers precise surface energy tailoring for advanced functional material printing.

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Area of Science:

  • Materials Science
  • Surface Chemistry
  • Nanotechnology

Background:

  • Substrate surface properties critically influence functional material printing resolution and stability.
  • Inkjet printing often faces wetting challenges on homogeneous substrates due to suboptimal surface characteristics.

Purpose of the Study:

  • To investigate methods for mediating substrate wetting and improving inkjet print quality.
  • To develop a precise technique for tailoring surface energy using thin polymeric layers.

Main Methods:

  • Deposition of nanometer-thick polymeric layers to modify surface energy and polarity.
  • Utilizing thermal decomposition of poly(methyl methacrylate) (PMMA) for controlled surface energy adjustment.
  • Evaluating wetting behavior across diverse substrate-ink systems.

Main Results:

  • Thin polymeric layers effectively mediate substrate wetting and enhance printed pattern quality.
  • PMMA layer thickness approaching zero facilitates smooth wetting transitions, likely via substrate surface percolation.
  • Successful adjustment of wetting was demonstrated for tantalum-oxide/indium-tin-oxide, lead zirconate titanate/platinized silicon, and silver nanoparticle/alumina systems.

Conclusions:

  • Nanometer-scale polymer coatings provide a versatile approach to control surface properties for inkjet printing.
  • Thermal decomposition of PMMA offers a precise and simple method for surface energy tailoring.
  • This technique enables high-resolution inkjet printing of complex structures on various functional materials.