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Updated: Feb 22, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Inline self-diffraction dispersion-scan of over octave-spanning pulses in the single-cycle regime
Abstract:
We present an implementation of dispersion-scan based on self-diffraction (SD d-scan) and apply it to the measurement of over octave-spanning sub-4-fs pulses. The results are compared with second-harmonic generation (SHG) d-scan. The efficiency of the SD process is derived theoretically and compared with the spectral response retrieved by the d-scan algorithm. The new SD d-scan has a robust inline setup and enables measuring pulses with over-octave spectra, single-cycle durations, and wavelength ranges beyond those of SHG crystals, such as the ultraviolet and the deep-ultraviolet.
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