Tailoring optical pulling force on gain coated nanoparticles with nonlocal effective medium theory

We study the optical scattering force on the coated nanoparticles with gain core and nonlocal plasmonic shell in the long-wavelength limit, and demonstrate negative optical force acting on the nanoparticles near the symmetric and/or antisymmetric surface plasmon resonances. To understand the optical force behavior, we propose nonlocal effective medium theory to derive the equivalent permittivity for the coated nanoparticles with nonlocality. We show that the imaginary part of the equivalent permittivity is negative near the surface resonant wavelength, resulting in the negative optical force. The introduction of nonlocality may shift the resonant wavelength of the optical force, and strengthen the negative optical force. Two examples of Fano-like resonant scattering in such coated nanoparticles are considered, and Fano resonance-induced negative optical force is found too. Our findings could have some potential applications in plasmonics, nano-optical manipulation, and optical selection.