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Origami Inspired Self-assembly of Patterned and Reconfigurable Particles
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Steering on-surface reactions with self-assembly strategy.

Xiong Zhou1, Jingxin Dai, Kai Wu

  • 1BNLMS, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China. kaiwu@pku.edu.cn.

Physical Chemistry Chemical Physics : PCCP
|November 25, 2017
PubMed
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Surface molecular assembly controls reactions by confining molecules, enabling precise steering of reaction pathways, sites, and selectivities for new surface chemistry applications.

Area of Science:

  • Surface Chemistry
  • Molecular Assembly
  • Reaction Engineering

Background:

  • Controlling molecular assembly is crucial for achieving desired functionalities.
  • Surface molecular assembly is explored for steering on-surface reactions.

Purpose of the Study:

  • To investigate surface molecular assembly as a strategy for controlling on-surface reactions.
  • To understand how assembly influences reaction selectivity, pathways, and sites.

Main Methods:

  • Utilizing assembly-assisted and assembly-involved reaction strategies.
  • Applying surface confinement effects to alter reaction dynamics.

Main Results:

  • Demonstrated that assembly strategies can effectively tweak reaction selectivities.

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  • Showcased the ability to steer reaction pathways and direct reaction sites through molecular assembly.
  • Identified surface confinement as a key principle affecting reaction energy barriers.

    • Conclusions:

    • Surface molecular assembly offers a powerful approach to control on-surface reactions.
    • This strategy can modify reaction dynamics by influencing the Arrhenius equation parameters.
    • Further development may unlock new routes for surface chemistry and single-molecule property manipulation.