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Enhanced Oxidation-Resistant Cu@Ni Core-Shell Nanoparticles for Printed Flexible Electrodes.

Tae Gon Kim1, Hye Jin Park1, Kyoohee Woo2

  • 1Division of Advanced Materials, Korea Research Institute of Chemical Technology (KRICT) , 141 Gajeongro, Daejeon 34114, Republic of Korea.

ACS Applied Materials & Interfaces
|December 12, 2017
PubMed
Summary

Highly conductive and stable copper-nickel (Cu@Ni) core-shell nanoparticle electrodes were fabricated on flexible polymer substrates. These electrodes show excellent performance for applications like flexible heaters, resisting harsh environmental conditions.

Keywords:
Cu nanoparticlecore−shell nanoparticleflexible electrodesflexible heaterphotonic sintering

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Area of Science:

  • Materials Science
  • Nanotechnology
  • Electrical Engineering

Background:

  • Developing robust and conductive electrodes for flexible electronics is crucial.
  • Existing materials often lack stability under environmental stress or require inert atmospheres for fabrication.

Purpose of the Study:

  • To fabricate and characterize highly conductive, flexible, and oxidation-resistant Cu-Ni core-shell nanoparticle (NP)-based electrodes.
  • To demonstrate the application of these electrodes in flexible heaters.

Main Methods:

  • Synthesis of Cu@Ni core-shell NPs with tunable nickel shell thickness via controlled Cu/Ni molar ratios.
  • Large-area conductor fabrication using continuous spray coating and flash photonic sintering in ambient atmosphere.
  • Electrode characterization including sheet resistance, stability testing (aging at 85°C/85% RH), and performance evaluation in a flexible heater.

Main Results:

  • Achieved low sheet resistance of 1.3 Ω sq⁻¹ with an optical energy dose of 1.5 J cm⁻².
  • Demonstrated high sheet resistance stability (ΔR/R₀ < 1) after 30 days of aging at 85°C/85% RH.
  • Fabricated a flexible heater with uniform heat distribution and stable temperature control using Cu@Ni films.

Conclusions:

  • Cu@Ni core-shell NPs offer a promising material for fabricating high-performance, stable electrodes on flexible substrates.
  • The ambient-processed Cu@Ni electrodes are suitable for demanding applications such as flexible heating elements.
  • This work presents a scalable method for producing advanced conductive materials for next-generation electronics.