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Conditional 1/f^{α} noise: From single molecules to macroscopic measurement.

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  • 1Department of Physics, Institute of Nanotechnology and Advanced Materials, Bar-Ilan University, Ramat-Gan 5290002, Israel.

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Single-molecule noise measurements reveal 1/f^{α} noise is nonstationary, unlike bulk measurements. This difference arises from the increasing number of fluctuating units over time, obscuring the true dynamics in macroscopic observations.

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Area of Science:

  • Physics
  • Physical Chemistry
  • Nanotechnology

Background:

  • Macroscopic measurements of 1/f^{α} noise often assume stationarity.
  • Single-molecule and nano-object dynamics can exhibit complex, time-dependent behavior.

Purpose of the Study:

  • To investigate the distinct characteristics of 1/f^{α} noise at the single-particle level compared to macroscopic measurements.
  • To elucidate the reasons behind the apparent stationarity observed in bulk measurements.

Main Methods:

  • Analysis of single-molecule and nano-object noise measurements.
  • Utilizing stochastic and deterministic models, including superimposed Lorentzians and blinking quantum dot models.
  • Exploring deterministic dynamics via nonlinear mapping.

Main Results:

  • Single-particle measurements of 1/f^{α} noise yield conditional time-dependent spectra.
  • Macroscopic measurements appear stationary due to an increasing number of fluctuating units over experimental timescales.
  • The inherent non-stationarity of 1/f^{α} spectra is masked in bulk measurements.

Conclusions:

  • 1/f^{α} noise at the single-particle level is fundamentally nonstationary.
  • Macroscopic averaging conceals the underlying time-dependent nature of single-unit fluctuations.
  • Understanding single-particle dynamics is crucial for interpreting complex noise phenomena.