Evaluation of particulate ¹³⁷Cs discharge from a mountainous forested catchment using reservoir sediments and sinking...

The time and size dependencies of particulate ¹³⁷Cs concentrations in a reservoir were investigated to evaluate the dynamics of ¹³⁷Cs pollution from a mountainous forested catchment. Sediment and sinking particle samples were collected using a vibracorer and a sediment trap at the Ogaki Dam Reservoir in Fukushima, which is located in the heavily contaminated area that formed as a result of the Fukushima Dai-ichi Nuclear Power Plant accident of 2011. The inventory of ¹³⁷Cs discharged into the reservoir during the post-accident period (965 days) was estimated to be approximately 3.0 × 10¹²-3.9 × 10¹² Bq, which is equivalent to 1.1%-1.4% of the initial estimated catchment inventory. The particulate ¹³⁷Cs concentration showed a decline with time, but the exponent value between the specific surface area and the ¹³⁷Cs concentration for the fine-sized (<63 μm) particle fraction remained almost constant from the immediate aftermath of the accident. These quantitative findings obtained by reconstructing the contamination history of particulate ¹³⁷Cs in reservoir sediments and sinking particles have important implications for the evaluation of ¹³⁷Cs dynamics in mountainous forested catchments.