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Quantized pseudomodes for plasmonic cavity QED.

Stephen Hughes, Marten Richter, Andreas Knorr

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    This summary is machine-generated.

    We developed a quantized pseudomode theory to analyze quantum systems with plasmonic resonators. This approach reveals new insights into multi-mode vacuum Rabi oscillations and population inversion phenomena in quantum electrodynamics.

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    Area of Science:

    • Quantum optics
    • Plasmonics
    • Cavity Quantum Electrodynamics

    Background:

    • Cavity Quantum Electrodynamics (CQED) describes light-matter interactions in confined electromagnetic fields.
    • Plasmonic resonators offer unique platforms for enhancing light-matter interactions at the nanoscale.

    Purpose of the Study:

    • To present a quantized pseudomode theory for system-level CQED involving quantum emitters and plasmonic resonators.
    • To investigate non-Markovian coupling regimes and multi-photon resonances in such systems.

    Main Methods:

    • Utilizing Green function response of a silver nanoparticle.
    • Applying an exact solution for input-output coupling.
    • Analyzing multi-mode vacuum Rabi oscillations and coherently pumped resonances.

    Main Results:

    • The theory accurately models non-Markovian coupling regimes.
    • Observed multi-mode vacuum Rabi oscillations and multi-photon resonances.
    • Demonstrated population inversion of a two-level atom via dark plasmon-dominated multiphoton resonances.

    Conclusions:

    • The quantized pseudomode theory provides a robust framework for studying complex CQED systems with plasmonics.
    • The findings highlight the role of collective plasmon modes and dark plasmons in achieving population inversion.