Spatiotemporal land use random forest model for estimating metropolitan NO₂ exposure in Japan

Adequate spatial and temporal estimates of NO₂ concentrations are essential for proper prenatal exposure assessment. Here, we develop a spatiotemporal land use random forest (LURF) model of the monthly mean NO₂ over four years in a metropolitan area of Japan. The overall objective is to obtain accurate NO₂ estimates for use in prenatal exposure assessments. We use random forests to convey the non-linear relationship between NO₂ concentrations and predictor variables, and compare the prediction accuracy with that of a linear regression. In addition, we include the distance decay effect of emission sources on NO₂ concentrations for more efficient model construction. The prediction accuracy of the LURF model is evaluated through a leave-one-monitor-out cross validation. We obtain a high R² value of 0.79, which is better than that of the conventional land use regression model using linear regression (R² of 0.73). We also evaluate the LURF model via a temporal and overall cross validation and obtain R² values of 0.84 and 0.92, respectively. We successfully integrate temporal and spatial components into our model, which exhibits higher accuracy than spatial models constructed individually for each month. Our findings illustrate the advantage of using a LURF to model the spatiotemporal variability of NO₂ concentrations.