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Magnetic Ground State Stabilized by Three-Site Interactions: Fe/Rh(111)
Andreas Krönlein1, Martin Schmitt1, Markus Hoffmann2
1Physikalisches Institut, Lehrstuhl für Experimentelle Physik 2, Universität Würzburg, Am Hubland, 97074 Würzburg, Germany.
Physical Review Letters
|June 5, 2018
Summary
Researchers directly observed a predicted magnetic ground state in a monolayer iron (Fe) film on Rhodium (Rh)(111). This exotic up-up-down-down spin structure confirms the role of complex spin interactions in thin magnetic films.
Area of Science:
- Surface Science
- Condensed Matter Physics
- Magnetism
Background:
- Monolayer magnetic films exhibit unique magnetic properties distinct from bulk materials.
- Theoretical models predicted exotic spin structures in iron (Fe) monolayers on Rhodium (Rh)(111).
Purpose of the Study:
- To directly observe the theoretically predicted magnetic ground state of a monolayer Fe on Rh(111).
- To investigate the role of higher-order spin interactions in itinerant magnets.
Main Methods:
- Spin-polarized scanning tunneling microscopy (SP-STM) was employed for direct imaging.
- Experiments utilized magnetic probe tips and external magnetic fields to probe spin structure.
Main Results:
- The study directly observed the up-up-down-down (↑↑↓↓) double-row-wise antiferromagnetic spin structure.
- This exotic phase was found to exist in three orientational domains.
- Evidence for a four-spin-three-site beyond-Heisenberg interaction contributing to spin coupling was found.
Conclusions:
- The experimental observation confirms the existence of the predicted ↑↑↓↓ magnetic order.
- The findings substantiate the significant contribution of higher-order, three-site interactions in thin magnetic films of itinerant magnets.
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