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A battery is a galvanic cell that is used as a source of electrical power for specific applications. Modern batteries exist in a multitude of forms to accommodate various applications, from tiny button batteries such as those that power wristwatches to the very large batteries used to supply backup energy to municipal power grids. Some batteries are designed for single-use applications and cannot be recharged (primary cells), while others are based on conveniently reversible cell reactions that...
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An ionic compound is stable because of the electrostatic attraction between its positive and negative ions. The lattice energy of a compound is a measure of the strength of this attraction. The lattice energy (ΔHlattice) of an ionic compound is defined as the energy required to separate one mole of the solid into its component gaseous ions. For the ionic solid sodium chloride, the lattice energy is the enthalpy change of the process:
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Crystalline solids are divided into four types: molecular, ionic, metallic, and covalent network based on the type of constituent units and their interparticle interactions.
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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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Metallic solids such as crystals of copper, aluminum, and iron are formed by metal atoms. The structure of metallic crystals is often described as a uniform distribution of atomic nuclei within a “sea” of delocalized electrons. The atoms within such a metallic solid are held together by a unique force known as metallic bonding that gives rise to many useful and varied bulk properties.
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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Monolithic All-Phosphate Solid-State Lithium-Ion Battery with Improved Interfacial Compatibility.

Shicheng Yu1, Andreas Mertens1, Hermann Tempel1

  • 1Institut für Energie- und Klimaforschung (IEK-9: Grundlagen der Elektrochemie) , Forschungszentrum Jülich , D-52425 Jülich , Germany.

ACS Applied Materials & Interfaces
|June 13, 2018
PubMed
Summary
This summary is machine-generated.

A novel all-phosphate solid-state battery demonstrates competitive cycling performance by optimizing interfacial matching between screen-printed electrodes and a solid electrolyte. This design enhances electrochemical stability and durability for advanced battery applications.

Keywords:
all-solid-state batteryinterfacial kineticslithium-ion batteryphosphatesolid electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • High interfacial resistance between solid electrolytes and electrodes hinders ceramic all-solid-state battery performance.
  • Developing stable and efficient interfaces is crucial for next-generation batteries.

Purpose of the Study:

  • To realize a monolithic all-phosphate solid-state battery with improved interfacial compatibility and cycling performance.
  • To investigate the impact of material selection and morphology on battery stability and efficiency.

Main Methods:

  • Fabrication of a solid-state battery using screen-printed LiTi2(PO4)3 anode and Li3V2(PO4)3 cathode on a Li1.3Al0.3Ti1.7(PO4)3 solid electrolyte.
  • Electrochemical characterization including cycling performance and impedance analysis.
  • Analysis of electrode/electrolyte interfaces using distribution of relaxation times.

Main Results:

  • Achieved a discharge capacity of 63.5 mAh g-1 at 0.39 C after 500 cycles (84% retention).
  • Demonstrated excellent electrochemical stability due to matched operating voltage and electrolyte window.
  • Confirmed stable electrode/electrolyte interfaces after cycling via impedance analysis.
  • The battery can be processed and operated in air due to low oxygen sensitivity of phosphate materials.

Conclusions:

  • The monolithic all-phosphate solid-state battery concept offers a viable strategy for high-performance energy storage.
  • Optimized interfacial engineering and material selection are key to overcoming limitations in solid-state batteries.
  • The developed battery exhibits promising durability and air processability for practical applications.