Enhanced Power Output of a Triboelectric Nanogenerator using Poly(dimethylsiloxane) Modified with Graphene Oxide and Sodium Dodecyl Sulfate

In this work, a new approach to modifying poly(dimethylsiloxane) (PDMS) as a negative triboelectric material using graphene oxide (GO) and a sodium dodecyl sulfate (SDS) surfactant was reported. A porous PDMS@GO@SDS composite triboelectric nanogenerator (TENG) could deliver an output voltage and current of up to 438 V and 11 μA/cm², respectively. These values were 3-fold higher than those of the flat PDMS. The superior performance is attributed to the intensified negative charges on PDMS from the oxygen functional groups of GO and anionic head groups of the SDS molecules. The outstanding performance and straightforward, low-cost fabrication process of the PDMS@GO@SDS TENG would be beneficial for the further development of powerful NGs integrated into wearable electronics and self-charging power cells.