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Related Concept Videos

Colloids03:22

Colloids

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Children at play often make suspensions such as mixtures of mud and water, flour and water, or a suspension of solid pigments in water known as tempera paint. These suspensions are heterogeneous mixtures composed of relatively large particles that are visible to the naked eye or can be seen with a magnifying glass. They are cloudy, and the suspended particles settle out after mixing. On the other hand, a solution is a homogeneous mixture in which no settling occurs and in which the dissolved...
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Colloids and Suspensions01:17

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Children at play often make suspensions such as mixtures of mud and water, flour and water, or a suspension of solid pigments in water known as tempera paint. These suspensions are heterogeneous mixtures composed of relatively large particles visible to the naked eye or seen with a magnifying glass. They are cloudy, and the suspended particles settle out after mixing. The suspended particles in a suspension settle out after some time of mixing. The separation of particles from a suspension is...
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The high insolubility of some precipitates can result in an unfavorable relative supersaturation. This can lead to colloidal particles with a large surface-to-mass ratio, where adsorption is promoted. For instance, in the precipitation of silver chloride, silver ions are adsorbed on the surface of the colloidal particles, forming a primary layer. This layer attracts ions of opposite charge (such as nitrate ions), forming a diffuse secondary layer of adsorbed ions. This electric double layer...
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Intrinsically Disordered Proteins02:18

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Intrinsically disordered proteins are a group of proteins that do not fold into specific three-dimensional structures. Their structural flexibility allows them to complement ordered proteins to perform functions that are inaccessible to rigid structures. They are more common in eukaryotes than prokaryotes and may either be exclusively intrinsically disordered or hybrid proteins, consisting of a mix of ordered and disordered regions. The absence of a rigid structure in these proteins can be...
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Bone Disorders01:29

Bone Disorders

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Aging and its effect on bone remodeling is the most common cause of bone disorders. In young and healthy people, bone deposition and resorption happen at an equal rate to maintain optimal bone health.
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Disorders of Erythrocytes01:27

Disorders of Erythrocytes

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Disorders of erythrocytes, or red blood cells (RBCs), include a range of conditions affecting their number, shape, or function.
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Synthesis and Characterization of Supramolecular Colloids
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Disorder Foreshadows Order in Colloidal Cubes.

Abhishek K Sharma1, Fernando A Escobedo1

  • 1Robert Frederick Smith School of Chemical and Biomolecular Engineering , Cornell University , Ithaca , New York 14853 , United States.

The Journal of Physical Chemistry. B
|September 7, 2018
PubMed
Summary

Colloidal hard cubes spontaneously form ordered domains in disordered states. These domains grow and merge, leading to a spontaneous phase transition without classical nucleation, influenced by pressure.

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Area of Science:

  • Physical chemistry
  • Materials science

Background:

  • Colloidal systems exhibit complex phase behavior.
  • Understanding disorder-to-order transitions is crucial for materials design.

Purpose of the Study:

  • Investigate the mechanism of the disorder-to-order phase transition in colloidal hard cubes.
  • Characterize the role of ordered domains in the transition process.

Main Methods:

  • Monte Carlo simulations were employed.
  • Analysis focused on spontaneous domain formation and growth.
  • A global order parameter was utilized.

Main Results:

  • Ordered domains appear transiently in the disordered phase due to entropic effects.
  • A classical nucleation process was not observed; domains percolate and consolidate.
  • Domain growth and critical pressure decrease with increasing system pressure.

Conclusions:

  • The transition is driven by the percolation and consolidation of pre-existing ordered domains.
  • A critical pressure exists above which spontaneous ordering occurs in large systems.
  • Interdomain zones actively mediate particle reorientation for monodomain formation.