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High-throughput micro-nanostructuring by microdroplet inkjet printing.

Hendrikje R Neumann1, Christine Selhuber-Unkel1

  • 1Biocompatible Nanomaterials, Institute for Materials Science, University of Kiel, Kaiserstr. 2, 24143 Kiel, Germany.

Beilstein Journal of Nanotechnology
|September 27, 2018
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Summary

Combining block copolymer micelle nanolithography with inkjet printing enables high-throughput fabrication of hierarchical gold nanoparticle microstructures. This method precisely controls nanoparticle patterns at the micrometer scale for diverse applications.

Keywords:
biofunctional surfacesinkjet printingmicrostructuresnanolithographynanoparticles

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Area of Science:

  • Materials Science
  • Nanotechnology
  • Surface Chemistry

Background:

  • Fabricating patterned nanoparticle structures is crucial for nano-optics, biosensors, and biomaterials.
  • Block copolymer micelle nanolithography creates nanoscale patterns but struggles with micrometer-scale hierarchical structures.
  • Existing methods lack efficiency in generating user-defined, large-scale nanoparticle arrangements.

Purpose of the Study:

  • To develop a high-throughput method for creating hierarchical micro-nanopatterns of gold nanoparticles.
  • To integrate inkjet printing with block copolymer micelle nanolithography for scalable patterning.
  • To investigate the influence of surface properties on nanoparticle arrangement.

Main Methods:

  • Utilized inkjet printing to deposit block copolymer micelle solutions onto various surfaces.
  • Employed block copolymer micelle nanolithography for self-assembly of gold nanoparticles within printed droplets.
  • Analyzed nanoparticle spacing and pattern formation on silicon and nickel-titanium substrates.

Main Results:

  • Achieved hierarchical patterns of gold nanoparticles with interparticle spacing of 25-42 nm.
  • Demonstrated high-throughput patterning with fabrication times of seconds.
  • Observed that surface material and topography influence the resulting nanoparticle patterns.
  • Successfully produced quasi-hexagonal micro-nanopatterns on smooth surfaces.

Conclusions:

  • The combined inkjet printing and block copolymer micelle nanolithography approach offers efficient, user-defined micrometer-scale patterning of nanoparticles.
  • This method is highly relevant for biological applications due to nanoparticle functionalization potential.
  • The technique provides a scalable solution for creating complex nanoparticle architectures on surfaces.