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Temperature-Driven Topological Phase Transition and Intermediate Dirac Semimetal Phase in ZrTe_{5}
1Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland.
Zirconium telluride (ZrTe5) undergoes a temperature-driven topological quantum phase transition. Infrared spectroscopy reveals a Dirac semimetal state at the transition, reconciling previous research on ZrTe5
Area of Science:
- Condensed matter physics
- Materials science
- Quantum materials
Background:
- Topological insulators (TIs) are materials with unique electronic properties.
- ZrTe5 has been theoretically proposed to host a topological quantum phase transition.
- Experimental verification of ZrTe5's topological nature remains debated.
Purpose of the Study:
- To experimentally investigate the topological phase transition in ZrTe5 using infrared spectroscopy.
- To determine the temperature dependence of the energy gap and electronic structure.
- To reconcile conflicting reports on the topological properties of ZrTe5.
Main Methods:
- Infrared spectroscopy was employed to study ZrTe5.
- The temperature evolution of the energy gap was analyzed.
- Optical conductivity was measured to identify signatures of a Dirac semimetal state.
Main Results:
- A temperature-driven topological quantum phase transition was confirmed in ZrTe5.
- An intermediate Dirac semimetal state was observed around Tp ≃ 138 K.
- The energy gap closes at the transition, and optical conductivity shows Dirac semimetal characteristics.
Conclusions:
- The study confirms the theoretical proposal of a topological quantum phase transition in ZrTe5.
- The observed Dirac semimetal state reconciles previous experimental discrepancies.
- The transition temperature (Tp) is sensitive to crystal growth conditions.
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