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Updated: Jan 29, 2026

Fabrication of Polymer Microspheres for Optical Resonator and Laser Applications
Published on: June 2, 2017
Unveiling lasing mechanism in CsPbBr3 microsphere cavities.
Wenna Du1, Shuai Zhang, Zhiyong Wu
1CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China. liuxf@nanoctr.cn.
This study reveals the lasing mechanism in CsPbBr3 perovskite microspheres, shifting from exciton-exciton to exciton-phonon scattering with increasing temperature. This finding is crucial for developing advanced low-threshold perovskite lasers.
Area of Science:
- Optics and Photonics
- Materials Science
- Condensed Matter Physics
Background:
- Perovskite microcavities show promise for low-threshold lasing devices.
- The precise lasing mechanisms in perovskites are not fully understood.
Purpose of the Study:
- To investigate the lasing mechanisms in CsPbBr3 microspheres.
- To elucidate the temperature-dependent behavior of light-matter interactions in perovskite microcavities.
Main Methods:
- Fabrication of high-quality CsPbBr3 microspheres.
- Temperature-dependent photoluminescence (PL) and time-resolved photoluminescence (TRPL) spectroscopy.
- Temperature-dependent Raman spectroscopy.
Main Results:
- Demonstrated single-mode excitonic lasing in CsPbBr3 microspheres.
- Identified a shift in lasing mechanism from exciton-exciton to exciton-phonon scattering between 77 K and 300 K.
- Revealed the involvement of two distinct phonon modes (8.6 meV and 15.3 meV) in exciton-phonon scattering, with dominance varying by temperature range.
Conclusions:
- The study clarifies the temperature-dependent lasing mechanisms in CsPbBr3 perovskite microcavities.
- Understanding these mechanisms is vital for the advancement of low-threshold perovskite lasers.

