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Polymer Electrolyte Glue: A Universal Interfacial Modification Strategy for All-Solid-State Li Batteries.

Derui Dong1, Bin Zhou1, Yufei Sun1

  • 1College of Materials Science and Engineering , Huaqiao University , Xiamen 361021 , China.

Nano Letters
|March 12, 2019
PubMed
Summary

A novel polymer glue electrolyte improves solid-state battery performance by enhancing electrode-electrolyte contact. This strategy significantly reduces interfacial resistance in lithium-ion and lithium-sulfur batteries, boosting stability and conductivity.

Keywords:
Polymer electrolyteglueinterfacesolid-state battery

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid lithium-ion conductors offer potential advantages over liquid electrolytes but face challenges.
  • High interfacial resistance between solid electrolytes and electrodes hinders practical battery applications.

Purpose of the Study:

  • To develop a universal strategy for modifying interfaces in solid-state batteries.
  • To reduce high interfacial resistance by improving solid-solid contact using a polymer glue electrolyte.

Main Methods:

  • Coating a curable polymer-based glue electrolyte between solid electrolyte and electrodes.
  • Utilizing the glue's wettability and stability, followed by post-curing to form a solid layer.
  • Testing symmetric lithium batteries and all-solid-state lithium-sulfur batteries with and without the glue modification.

Main Results:

  • Glue modification significantly decreased impedance in symmetric lithium batteries.
  • Enhanced stability was observed in plating/stripping cycles for modified batteries.
  • All-solid-state lithium-sulfur batteries demonstrated significantly improved performance with glue modification.

Conclusions:

  • The polymer glue electrolyte effectively addresses poor solid-solid contact, reducing interfacial resistance.
  • This interfacial modification strategy offers a promising approach for enhancing solid-state battery performance.
  • The developed glue electrolyte technique is applicable to various solid-state battery chemistries.