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An All-Solid-State Rechargeable Chloride Ion Battery.

Chao Chen1, Tingting Yu1, Meng Yang1

  • 1College of Materials Science and Engineering Jiangsu Collaborative Innovation Center for Advanced Inorganic Functional Composites Nanjing Tech University Nanjing 211816 China.

Advanced Science (Weinheim, Baden-Wurttemberg, Germany)
|April 3, 2019
PubMed
Summary
This summary is machine-generated.

Researchers developed the first all-solid-state rechargeable chloride ion battery. This innovation uses a novel solid polymer electrolyte to overcome limitations of liquid electrolytes, enabling stable performance for chloride batteries.

Keywords:
chloride ion batterieselectrochemistryiron oxychloridepolymer electrolytesrechargeable batteries

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Chloride ion batteries offer an alternative to lithium-ion technology, utilizing abundant materials and promising high energy density.
  • Current chloride ion battery applications are hindered by electrode material dissolution and side reactions in liquid electrolytes.

Purpose of the Study:

  • To develop a stable solid polymer electrolyte for chloride ion transfer.
  • To demonstrate the feasibility of an all-solid-state rechargeable chloride ion battery.

Main Methods:

  • A solid polymer electrolyte was synthesized using poly(ethylene oxide), tributylmethylammonium chloride, and succinonitrile.
  • The electrolyte's conductivity was measured across a temperature range (298–343 K).
  • An all-solid-state battery was assembled using the developed electrolyte and an iron oxychloride/lithium electrode system.

Main Results:

  • The solid polymer electrolyte exhibited conductivities in the range of 10-5–10-4 S cm-1.
  • Reversible electrochemical redox reactions were observed at both the cathode (FeOCl/FeO) and anode (Li/LiCl) interfaces.
  • The successful assembly and operation of the first all-solid-state rechargeable chloride ion battery were demonstrated.

Conclusions:

  • The developed solid polymer electrolyte effectively facilitates chloride ion transfer and enhances battery stability.
  • This work presents a significant advancement towards practical and sustainable chloride ion battery technology.
  • The findings pave the way for future research in solid-state electrolytes for next-generation energy storage systems.