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Toward ideal carbon dioxide functionalization.

Yang Yang1, Ji-Woong Lee1

  • 1Department of Chemistry , University of Copenhagen , Universitetsparken 5 , Copenhagen Ø , 2100 , Denmark .

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Summary
This summary is machine-generated.

This perspective explores sustainable carbon dioxide (CO2) utilization in forming carbon-carbon bonds. Recent advances focus on catalytic CO2 functionalization under ambient conditions, overcoming CO2

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Area of Science:

  • * Sustainable chemistry and catalysis.
  • * Green chemistry and synthetic organic chemistry.

Background:

  • * Carbon dioxide (CO2) is kinetically inert and thermodynamically stable, posing challenges for its utilization.
  • * Current CO2 utilization methods often require energy-intensive conditions (high pressure/temperature) and reactive substrates, limiting broad applications.
  • * Recent research aims for catalytic CO2 utilization under ambient conditions, but is restricted in activation modes and substrate scope.

Purpose of the Study:

  • * To review recent advancements in sustainable carbon dioxide functionalization for carbon-carbon bond formation.
  • * To highlight ideal CO2 functionalization strategies emphasizing sustainability and practical synthetic applications.
  • * To discuss progress in metal-catalyzed, photochemical, redox-neutral, and enantioselective CO2 utilization.

Main Methods:

  • * Review of recent literature on catalytic CO2 utilization in C-C bond formation.
  • * Analysis of metal-catalyzed reductive carboxylation of halides, olefins, and allyl alcohols.
  • * Discussion of photochemical CO2 utilization, redox-neutral functionalization, and enantioselective catalysis for C-CO2 bond formation.

Main Results:

  • * Progress in metal-catalyzed reductive carboxylation reactions.
  • * Developments in photochemical and redox-neutral CO2 functionalization strategies.
  • * Emerging enantioselective catalysis for CO2 incorporation into C-CO2 bonds.

Conclusions:

  • * Sustainable CO2 functionalization is advancing, with a focus on ambient conditions and broader substrate scope.
  • * Redox-neutral, umpolung, and asymmetric carboxylation strategies are key for future ideal CO2 functionalization.
  • * Further development is needed to achieve general and efficient CO2 utilization in synthetic chemistry.